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Streszczenie:
Concrete shielding structures in nuclear facilities must maintain both radiation attenuation capacity and transport barrier performance throughout their service life. Although gas permeability and radiation shielding properties have been widely investigated, their coupled evolution under load-induced damage remains insufficiently understood, particularly for concretes with low-clinker cements. This study evaluates the combined effects of low-clinker cement type, aggregate type, and mechanical preloading on the gas permeability and gamma-ray shielding performance of concretes intended for nuclear applications. Six mixtures were produced using CEM II/C-M (V–F–LL) and CEM V/A (S–V) cements combined with magnetite, basalt or limestone aggregates. Gas permeability was measured using the Cembureau method on specimens subjected to progressive preloading up to 90% of the splitting tensile strength. Gamma-ray attenuation parameters were determined using a 137Cs source (0.662 MeV), and microstructural observations were performed by SEM. Aggregate type was the dominant factor governing shielding performance. Magnetite concretes exhibited the highest compressive strength, the lowest gas permeability, and the highest attenuation coefficients, reaching μ = 0.258 cm⁻¹ and HVL = 2.68 cm. CEM V concretes generally showed lower permeability than the corresponding CEM II concretes. Mechanical preloading increased gas permeability, particularly above approximately 80% of the splitting tensile strength, indicating the formation of connected microcrack networks. Simultaneously, a reduction in attenuation factor was observed, demonstrating that load-induced damage adversely affected shielding effectiveness. A relationship between the increase in permeability and the reduction in attenuation factor was identified, suggesting a transition from pore-controlled to crack-controlled behaviour. The results demonstrate the suitability of concretes with low-clinker cements for shielding applications and provide new insight into the coupling between damage development, transport properties, and radiation shielding performance.

Słowa kluczowe:
Permeability, Shielding concreto, Load, Microstructure, Low-clinker cement, Gamma-ray attenuation, Microcracking

Streszczenie:
The present study contributes to the development of alternative materials for radiation shielding, focusing on environmental sustainability and material cost efficiency. The primary aim was to evaluate the compressive and flexural strength, mineral composition, microstructure, and gamma-ray attenuation properties of cement mortars and geopolymer mortars containing barite powder. Mortars based on ordinary Portland cement (OPC) and fly ash geopolymers with varying amounts of barite powder were assessed for their shielding properties at energy levels associated with the decay of 137Cs. From the results, key parameters such as the linear attenuation coefficient (μ), mass attenuation coefficient (μm), half-value layer (HVL), and tenth-value layer (TVL) were determined. The results showed that while cement-based composites exhibited superior gamma radiation attenuation compared to fly ash geopolymer mortars, the latter had higher mass attenuation efficiency, meaning less material density was required for the same level of shielding. Additionally, cement mortars had 23–25 % higher mechanical strength than geopolymer mortars. Importantly, the inclusion of barite powder improved the radiation shielding performance of both materials by 7–10 %, demonstrating its effectiveness in enhancing the protective properties of these mortars. This research highlights the potential of fly ash geopolymer mortars as viable, eco-friendly alternatives to traditional cement mortars in radiation shielding applications.

Słowa kluczowe:
Cement mortar, Fly ash geopolymer mortar, Barite, Gamma ray attenuation, Microstructure

Streszczenie:
Concrete used in nuclear applications faces significant durability challenges due to degradation from radiation, thermal stresses, and chemical reactions. These issues highlight the critical need for impermeable concrete shields to prevent radioactive leaks and protect against harmful radiation. This study examines how concrete composition affects gas permeability and gamma radiation shielding properties. Three coarse aggregates—amphibolite (reference), magnetite, and serpentine—and two cement types (ordinary and slag) were tested, with concrete densities ranging from 2309 to 3538 kg/m3. Gas permeability was measured using a Cembureau-type constant head permeameter, and gamma shielding was assessed through the linear attenuation coefficient (µ) and half-value layer (HVL) at 137Cs decay energies. The results revealed significant variations in gas permeability and gamma ray shielding based on aggregate and cement type, with observable relationships between gas permeability, HVL, and concrete density. The results obtained from the presented research will contribute to increasing the safety, durability and cost-effectiveness of concrete constructions and maintenance of nuclear facilities.

Słowa kluczowe:
Heavyweight aggregate, Hydrogen-bearing aggregate, Shielding concrete, Gas permeability, Gamma ray attenuation, Microstructure, ITZ